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Redox biocatalysis : fundamentals and applications /
Increasingly, researchers rely on the use of enzymes to perform redox processes as they search for novel industrial synthetic routes. In order to support and advance their investigations, this book provides a comprehensive and current overview of the use of redox enzymes and enzyme-mediated oxidativ...
| Clasificación: | Libro Electrónico |
|---|---|
| Otros Autores: | |
| Formato: | Electrónico eBook |
| Idioma: | Inglés |
| Publicado: |
Hoboken, New Jersey :
Wiley,
©2012.
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| Temas: | |
| Acceso en línea: | Texto completo |
MARC
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| 245 | 0 | 0 | |a Redox biocatalysis : |b fundamentals and applications / |c Daniela Gamenara [and others]. |
| 260 | |a Hoboken, New Jersey : |b Wiley, |c ©2012. | ||
| 300 | |a 1 online resource | ||
| 336 | |a text |b txt |2 rdacontent | ||
| 337 | |a computer |b c |2 rdamedia | ||
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| 504 | |a Includes bibliographical references and index. | ||
| 588 | 0 | |a Print version record and CIP data provided by publisher. | |
| 520 | |a Increasingly, researchers rely on the use of enzymes to perform redox processes as they search for novel industrial synthetic routes. In order to support and advance their investigations, this book provides a comprehensive and current overview of the use of redox enzymes and enzyme-mediated oxidative processes, with an emphasis on the role of redox enzymes in chemical transformations. The authors examine the full range of topics in the field, from basic principles to new and emerging research and applications. Moreover, they explore everything from laboratory-scale procedures to industrial manufacturing. Redox Biocatalysis begins with a discussion of the biochemical features of redox enzymes as well as cofactors and cofactor regeneration methods. Next, the authors present a variety of topics and materials to the research and development of full-scale industrial applications, including: Biocatalytic applications of redox enzymes such as dehydrogenases, oxygenases, oxidases, and peroxidases Enzyme-mediated oxidative processes based on biocatalytic promiscuity. All the steps from enzyme discovery to robust industrial processes, including directed evolution, high-throughput screening, and medium engineering. Case studies tracing the development of industrial applications using biocatalytic redox reactions. Each chapter ends with concluding remarks, underscoring the key scientific principles and processes. Extensive references serve as a gateway to the growing body of research in the field. Researchers in both academia and industry will find this book an indispensable reference for redox biotransformations, guiding them from underlying core principles to new discoveries and emerging industrial applications. | ||
| 505 | 0 | |a REDOX BIOCATALYSIS; CONTENTS; PREFACE; 1. Enzymes Involved in Redox Reactions: Natural Sources and Mechanistic Overview; 1.1 Motivation: Green Chemistry and Biocatalysis; 1.2 Sources of Biocatalysts; 1.2.1 Plants and Animals as Sources of Redox Biocatalysts; 1.2.2 Wild-Type Microorganisms; 1.2.2.1 Yeasts; 1.2.2.2 Fungi; 1.2.2.3 Bacteria; 1.2.3 Metagenomic Assessments; 1.3 Overview of Redox Enzymes; 1.3.1 Dehydrogenases; 1.3.1.1 Zn-Dependent Dehydrogenases; 1.3.1.2 Flavin-Dependent Dehydrogenases; 1.3.1.3 Pterin-Dependent Dehydrogenases; 1.3.1.4 Quinoprotein Dehydrogenases | |
| 505 | 8 | |a 1.3.1.5 Dehydrogenases without Prosthetic Group1.3.2 Oxygenases; 1.3.2.1 Monooxygenases; 1.3.2.2 Dioxygenases; 1.3.3 Oxidases; 1.3.3.1 Iron-Containing Oxidases; 1.3.3.2 Copper-Containing Oxidases; 1.3.3.3 Flavin-Dependent Oxidases; 1.3.4 Peroxidases; 1.4 Concluding Remarks; References; 2. Natural Cofactors and Their Regeneration Strategies; 2.1 Types of Natural Cofactors-Mechanisms; 2.2 Cofactor Regeneration; 2.2.1 Enzymatic Regeneration of Reduced Cofactors; 2.2.1.1 Substrate-Assisted Method; 2.2.1.2 Enzyme-Assisted Method; 2.2.2 Enzymatic Regeneration of Oxidized Cofactors | |
| 505 | 8 | |a 3.7 Dehydrogenase-Catalyzed Redox Reactions in Natural Products3.8 Concluding Remarks; References; 4. Reactions Involving Oxygenases; 4.1 Monooxygenase-Catalyzed Reactions; 4.1.1 Hydroxylation of Aliphatic Compounds; 4.1.2 Hydroxylation of Aromatic Compounds; 4.1.3 Baeyer-Villiger Reactions; 4.1.3.1 Classification and Metabolic Role of BVMOs; 4.1.3.2 Isolated Enzymes versus Whole-Cell Systems (Wild-Type and Recombinant Microorganisms); 4.1.3.3 Substrate Profile of Available Baeyer-Villiger Monooxygenases; 4.1.3.4 Synthetic Applications of BVMOs; 4.1.4 Epoxidation of Alkenes | |
| 505 | 8 | |a 4.2 Dioxygenase-Catalyzed Reactions4.2.1 Aromatic Dioxygenases; 4.2.1.1 Dihydroxylation of Aromatic Compounds; 4.2.1.2 Other Oxidation Reactions Performed by Aromatic Dioxygenases; 4.2.2 Miscellaneous Dioxygenases; 4.2.2.1 Lipoxygenase; 4.3 Concluding Remarks; References; 5. Reactions Involving Oxidases and Peroxidases; 5.1 Oxidase-Catalyzed Reactions; 5.1.1 Oxidases Acting on C-O Bonds; 5.1.1.1 Galactose Oxidase; 5.1.1.2 Pyranose Oxidase; 5.1.1.3 Alcohol Oxidase; 5.1.1.4 Glucose Oxidase; 5.1.1.5 Glycolate Oxidase; 5.1.2 Laccases and Tyrosinases (Phenol Oxidases); 5.1.2.1 Laccase | |
| 590 | |a ProQuest Ebook Central |b Ebook Central Academic Complete | ||
| 650 | 0 | |a Environmental chemistry. | |
| 650 | 0 | |a Green chemistry. | |
| 650 | 0 | |a Oxidation-reduction reaction. | |
| 650 | 0 | |a Enzymes. | |
| 650 | 6 | |a Chimie de l'environnement. | |
| 650 | 6 | |a Chimie verte. | |
| 650 | 6 | |a Oxydoréduction. | |
| 650 | 6 | |a Enzymes. | |
| 650 | 7 | |a enzyme. |2 aat | |
| 650 | 7 | |a SCIENCE |x Biotechnology. |2 bisacsh | |
| 650 | 7 | |a Environmental chemistry |2 fast | |
| 650 | 7 | |a Enzymes |2 fast | |
| 650 | 7 | |a Green chemistry |2 fast | |
| 650 | 7 | |a Oxidation-reduction reaction |2 fast | |
| 700 | 1 | |a Gamenara, Daniela, |d 1964- |1 https://id.oclc.org/worldcat/entity/E39PCjFpc7KjQPkvrJxyPT3pHd | |
| 758 | |i has work: |a Redox biocatalysis (Text) |1 https://id.oclc.org/worldcat/entity/E39PCGYH6FJCydQDQ6CtJJ4JcP |4 https://id.oclc.org/worldcat/ontology/hasWork | ||
| 776 | 0 | 8 | |i Print version: |t Redox biocatalysis. |d Hoboken, N.J. : Wiley, ©2012 |z 9780470874202 |w (DLC) 2012025734 |
| 856 | 4 | 0 | |u https://ebookcentral.uam.elogim.com/lib/uam-ebooks/detail.action?docID=918272 |z Texto completo |
| 880 | 0 | |6 505-00/(S |a REDOX BIOCATALYSIS -- CONTENTS -- PREFACE -- 1. Enzymes Involved in Redox Reactions: Natural Sources and Mechanistic Overview -- 1.1 Motivation: Green Chemistry and Biocatalysis -- 1.2 Sources of Biocatalysts -- 1.2.1 Plants and Animals as Sources of Redox Biocatalysts -- 1.2.2 Wild-Type Microorganisms -- 1.2.2.1 Yeasts -- 1.2.2.2 Fungi -- 1.2.2.3 Bacteria -- 1.2.3 Metagenomic Assessments -- 1.3 Overview of Redox Enzymes -- 1.3.1 Dehydrogenases -- 1.3.1.1 Zn-Dependent Dehydrogenases -- 1.3.1.2 Flavin-Dependent Dehydrogenases -- 1.3.1.3 Pterin-Dependent Dehydrogenases -- 1.3.1.4 Quinoprotein Dehydrogenases -- 1.3.1.5 Dehydrogenases without Prosthetic Group -- 1.3.2 Oxygenases -- 1.3.2.1 Monooxygenases -- 1.3.2.2 Dioxygenases -- 1.3.3 Oxidases -- 1.3.3.1 Iron-Containing Oxidases -- 1.3.3.2 Copper-Containing Oxidases -- 1.3.3.3 Flavin-Dependent Oxidases -- 1.3.4 Peroxidases -- 1.4 Concluding Remarks -- References -- 2. Natural Cofactors and Their Regeneration Strategies -- 2.1 Types of Natural Cofactors-Mechanisms -- 2.2 Cofactor Regeneration -- 2.2.1 Enzymatic Regeneration of Reduced Cofactors -- 2.2.1.1 Substrate-Assisted Method -- 2.2.1.2 Enzyme-Assisted Method -- 2.2.2 Enzymatic Regeneration of Oxidized Cofactors -- 2.2.3 Chemical Regeneration of Cofactors -- 2.2.4 Electrochemical Regeneration of Cofactors -- 2.2.5 Photochemical Regeneration of Cofactors -- 2.3 Concluding Remarks -- References -- 3. Reactions Involving Dehydrogenases -- 3.1 General Considerations -- 3.2 Reduction of Carbonyl Groups -- 3.2.1 Reduction of Aliphatic and Aromatic Ketones -- 3.2.2 Reduction of α- and β-keto Esters and Derivatives -- 3.2.3 Reduction of Diketones -- 3.2.4 Reduction of Aldehydes -- 3.3 Racemization and Deracemization Reactions -- 3.4 Preparation of Amines -- 3.5 Reduction of C-C Double Bonds -- 3.6 Oxidation Reactions. | |
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