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XUV Pump-Probe Experiments on Diatomic Molecules Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay /

This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is s...

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Detalles Bibliográficos
Clasificación:Libro Electrónico
Autor principal: Schnorr, Kirsten (Autor)
Autor Corporativo: SpringerLink (Online service)
Formato: Electrónico eBook
Idioma:Inglés
Publicado: Cham : Springer International Publishing : Imprint: Springer, 2015.
Edición:1st ed. 2015.
Colección:Springer Theses, Recognizing Outstanding Ph.D. Research,
Temas:
Acceso en línea:Texto Completo

MARC

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245 1 0 |a XUV Pump-Probe Experiments on Diatomic Molecules  |h [electronic resource] :  |b Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay /  |c by Kirsten Schnorr. 
250 |a 1st ed. 2015. 
264 1 |a Cham :  |b Springer International Publishing :  |b Imprint: Springer,  |c 2015. 
300 |a XI, 191 p. 95 illus., 25 illus. in color.  |b online resource. 
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490 1 |a Springer Theses, Recognizing Outstanding Ph.D. Research,  |x 2190-5061 
505 0 |a Introduction -- Photoionization and Interatomic Coulombic Decay -- Free-Electron Lasers -- Experimental Setup -- Data Analysis -- Ionization Dynamics of I2 in XUV and IR Laser Pulses -- ICD Lifetime in Ne2 -- Conclusions and Outlook -- Appendices. 
520 |a This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is studied in an experiment that made it possible to access charge transfer in a thus far unexplored quasimolecular regime relevant for plasma and chemistry applications of the FEL. Secondly the lifetime of an efficient non-radiative relaxation process that occurs in weakly bound systems is measured directly for the first time in a neon dimer (Ne2). Interatomic Coulombic decay (ICD) has been identified as the dominant decay mechanism in inner-valence-ionized or excited van-der-Waals and hydrogen bonded systems, the latter being ubiquitous in all biomolecules. The role of ICD in DNA damage thus demands further investigation, e.g. with regard to applications like radiation therapy. 
650 0 |a Atoms. 
650 0 |a Molecules. 
650 0 |a Electrodynamics. 
650 0 |a Spectrum analysis. 
650 0 |a Medical physics. 
650 1 4 |a Atoms and molecules in external fields. 
650 2 4 |a Classical Electrodynamics. 
650 2 4 |a Spectroscopy. 
650 2 4 |a Medical Physics. 
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776 0 8 |i Printed edition:  |z 9783319121406 
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950 |a Physics and Astronomy (SpringerNature-11651) 
950 |a Physics and Astronomy (R0) (SpringerNature-43715)